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I really want Theatrhythm Final Fantasy for 3DS only, as it looks really good.
Also, if you like Pokémon, go for Pokémon Conquest; it's a mix of Pokémon and Nobunaga's Ambition (the Japanese side of Warriors Orochi and star of the Samurai Warriors series which are both made by Koei), a pretty perfect combination
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i'm looking forward to trying out kingdom hearts 3ds, i'm a huge fan of the series and i have high hopes! also thinking of getting pokemon conquest, which i hope is basically final fantasy tactics but with pokemon.
if you're also looking for old ds games i'd personally recommend games like the world ends with you, phoenix wright, the mario and luigi games.
mario 3d land is pretty neat and i'm super excited for paper mario sticker star later this year!
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Mario 3D Land is really fun, I re-bought New Super Mario Brothers after I played it, just for more Mario. I think New Super Mario Brothers 2 comes out on the 17th, it should be good too.
Also, I really like LOZ: Ocarina of Time 3D, just love that game, it's nice to have it in 3D/handheld.